Exploring Nuclear Fuels at High Pressure and Temperature: From Cradle to Grave

Actinide materials are of great importance due to their wide-ranging uses in modern industry.

October 1, 2021

Placeholder Image
Placeholder Image

Actinide materials are of great importance due to their wide-ranging uses in modern industry. For example, uranium dioxide (UO2) is used as the primary nuclear fuel in light-water reactors (LWRs). However, nuclear reactor accidents such as the Fukushima disaster in 2011 have encouraged the nuclear energy industry to explore alternative accident-tolerant nuclear fuels (ATNFs) such as uranium-silicide (U-Si) compounds. A number of U-Si phases (e.g., U3Si2, U3Si5) possess higher thermal conductivities than the conventional UO2 fuel under nuclear reactor operating conditions. Higher thermal conductivities allow better heat dissipation in ATNFs when used in reactors. Nonetheless, significant research is needed to understand their structural stability and physical properties (e.g., mechanical properties) under both ambient conditions and those of elevated pressures and temperatures. An important elastic property significant to ATNF mechanical integrity is compress-ibility (i.e., inverse of bulk modulus). A powerful tool to study mechanical properties is applied pressure due to its ability to change structural characteristics. By applying pressure in concert with X-ray diffraction (XRD) technique, structural behavior and mechanical strength can be examined.

Read the full article

Share
More In This Issue
Nuclear Thermal Rocket Reactors and Engine Systems: A RetrospectiveProbing the “Hidden Order” in Uranium Ruthenium SilicideRapid Measurements of Actinide Isotope Ratios in Nuclear MaterialsAll Stories

More Actinide Research Quarterly (ARQ) Stories

Actinide Research Quarterly (ARQ) Home
Cover Nuc Therm2x Opt 1cc87 Card

Nuclear Thermal Rocket Reactors and Engine Systems: A Retrospective

From the late 1950s to the early 1970s a major US program successfully developed the capability to conduct space exploration using the advanced technology of nuclear rocket propulsion.

Probing The “hidden Order2x Opt Ea0f6 Card

Probing the “Hidden Order” in Uranium Ruthenium Silicide

Understanding the behavior of actinide materials is important for issues such as developing new technology and predicting the aging of our nation’s nuclear stockpile.

Pu Isotopes2x Opt D9eed Card

Rapid Measurements of Actinide Isotope Ratios in Nuclear Materials

In order to properly characterize nuclear waste and perform nuclear forensics, we use an array of chemical tools.

Small Scale2x Opt B22d0 Card

Small-Scale Mechanical Testing of Actinide Compounds

Nuclear reactors produce 20% of the electrical power in the United States and represent a viable carbon-reducing energy source for future electrical production.

Topologicalphases2x Opt A0bb4 Card

Searching for Topological Phases in Lanthanide and Actinide Compounds

Ordered states of matter have traditionally been categorized by their broken symmetries, such as the loss of symmetry when spins order in a ferromagnet or liquid freezes into a crystalline solid.